原创力文档effect of current density on thermodynamic properties of nanocrystalline palladium capped samarium hydride thin film switchable mirrors电流密度对纳米晶体的热力学性质的影响限制钐钯氢化物薄膜可切换的镜子.pdfVIP
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effect of current density on thermodynamic properties of nanocrystalline palladium capped samarium hydride thin film switchable mirrors电流密度对纳米晶体的热力学性质的影响限制钐钯氢化物薄膜可切换的镜子
Hindawi Publishing Corporation
Journal of Nanomaterials
Volume 2007, Article ID 52083, 7 pages
doi:10.1155/2007/52083
Research Article
Effect of Current Density on Thermodynamic Properties of
Nanocrystalline Palladium Capped Samarium Hydride Thin
Film Switchable Mirrors
Pushpendra Kumar1, 2 and L. K. Malhotra2
1 Technische Physik, Universitat des Saarlandes, Geb. 38, Postfach 151150, 66041 Saarbrucken, Germany
¨ ¨
2 Thin Film Laboratory, Department of Physics, Indian Institute of Technology, Hauz Khas, New Delhi 110016, India
Received 20 November 2006; Accepted 12 December 2006
Recommended by Rakesh K. Joshi
A 55 nm samarium film capped with a 10 nm palladium overlayer switched from a metallic reflecting to a semiconducting, trans-
parent in visible state during ex-situ hydrogen loading via electrochemical means in 1 M KOH electrolytic aqueous solution at
room temperature. The switching between metal to semiconductor was accompanied by measurement of transmittance during
hydrogen loading/unloading. The effect of current density on switching and thermodynamic properties was studied between di-
hydride state (FCC phase) and trihydride state (hexagonal phase). From the plateau of partial pressure of hydrogen at x = 2.6,
enthalpy of formation was calculated at different current densities. The diffusion coefficients and switching kinetics are shown to
depend on applied current density.
Copyright © 2007 P. Kumar and L. K. Malhotra. This is an open access article distributed under the Creative Commons
Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is
properly cited.
1. INTRODUCTION
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