原创力文档selective sorption of dissolved organic carbon compounds by temperate soils由温带土壤溶解有机碳化合物的选择性吸附.pdfVIP
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selective sorption of dissolved organic carbon compounds by temperate soils由温带土壤溶解有机碳化合物的选择性吸附
Selective Sorption of Dissolved Organic Carbon
Compounds by Temperate Soils
Sindhu Jagadamma*, Melanie A. Mayes, Jana R. Phillips
Climate Change Science Institute and Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee, United States of America
Abstract
Background: Physico-chemical sorption onto soil minerals is one of the major processes of dissolved organic carbon (OC)
stabilization in deeper soils. The interaction of DOC on soil solids is related to the reactivity of soil minerals, the chemistry of
sorbate functional groups, and the stability of sorbate to microbial degradation. This study was conducted to examine the
sorption of diverse OC compounds (D-glucose, L-alanine, oxalic acid, salicylic acid, and sinapyl alcohol) on temperate
climate soil orders (Mollisols, Ultisols and Alfisols).
Methodology: Equilibrium batch experiments were conducted using 0–100 mg C L21 at a solid-solution ratio of 1:60 for
48 hrs on natural soils and on soils sterilized by c-irradiation. The maximum sorption capacity, Qmax and binding coefficient,
k were calculated by fitting to the Langmuir model.
Results: Ultisols appeared to sorb more glucose, alanine, and salicylic acid than did Alfisols or Mollisols and the isotherms
followed a non-linear pattern (higher k). Sterile experiments revealed that glucose and alanine were both readily degraded
and/or incorporated into microbial biomass because the observed Qmax under sterile conditions decreased by 22–46% for
glucose and 17–77% for alanine as compared to non-sterile conditions. Mollisols, in contrast, more readily reacted with
oxalic acid (Qmax of 886 mg kg21) and sinapyl alcohol (Qmax of 2031 mg kg21), and no degradation was observed. The
reactivity of Alfisols to DOC was intermediate to that of Ultisols and Mollisols, and degradation followed sim
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