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the role of isolated sites in heterogeneous catalysis characterization and modeling孤立的网站在多相催化特性和建模
Int. J. Mol. Sci. 2001, 2, 167-182
International Journal of
Molecular Sciences
ISSN 1422-0067
© 2001 by MDPI
/ijms/
The Role of Isolated Sites in Heterogeneous Catalysis:
Characterization and Modeling
Silvia Bordiga,1,2* Alessandro Damin,1,2 Gloria Berlier,1,2 Francesca Bonino,1,2 Gabriele Ric-
chiardi,1,2 Adriano Zecchina,1,2 and Carlo Lamberti1,2,3
1Department of Inorganic, Physical and Material Chemistry, University of Turin, Via P. Giuria 7
10125 Torino Italy.
2INSTM Research unit of Turin University
3INFM UdR di Torino Università
Tel.: (+39-011-6707858, Fax: +39-011 E-mail: Bordiga@ch.unito.it
*Author to whom correspondence should be addressed E-mail: Bordiga@ch.unito.it.
Received: 2 October 2001 / Accepted: 7 November 2001 / Published: 13 November 2001
Abstract: TS-1 and Fe-MFI systems have been chosen as cases studies for describing the
behavior of single-site catalysts. We will report a concise review of the firmly established
knowledge and of the open problems concerning the structure and the reactivity of Ti and
Fe sites in TS-1 and Fe-MFI in partial oxidation catalysts. Some new experimental and
theoretical results will also be described.
Keywords: single-site catalyst, oxidation catalysis, TS-1, Fe-MFI
1. Introduction
In recent years, two interesting classes single site catalysts active in partial oxidation reactions have
attracted particular interest in the scientific community i.e: i) the TS-1 [1-8] a
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