fenton氧化——絮凝法处理含毒害污染物废水的分析word格式论文.docx

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2018-05-18 发布于上海
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fenton氧化——絮凝法处理含毒害污染物废水的分析word格式论文.docx

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fenton氧化——絮凝法处理含毒害污染物废水的分析word格式论文

AbstractFentonoxidationprocessintreatingorganicsewageisadvanced,especiallycoupledwithflocculation.ThestrongoxidizingpropertyofFenton,adsorptioneffectofFe(OH)3andflocculationofpolymericflocculantcangreatlyreducetoxicandharmfulorganicpollutants.ThearticlewasbasedontreatingsewagewithPFOSandharmfulhydroquinoneinit.TheorganicwastewaterwasprocessedwithFentonandsedimentation.Differentfactorsweretestedintheprocessofreducingpollutants,such asreaction time,temperature,initialpHvalue,inputamountofH2O2,initialconcentrationofFe2+,salinityandflocculantadded.Conclusionsarelistedasfollows:FentonhadnooxidizationeffectonPFOS.Ifbasewasadded,thereaction productFe(OH)3couldadsorbPFOS,whoseconcentrationwouldbereducedto0.807mg·L-1 andreductionratewasalmost60%.Highsalinitycouldpromotetheadsorptioneffect.FlocculantCPAMcouldnoteliminatePFOSandaccelerate flocculation.The bestoperatingconditionforFenton tooxidizehydroquinone were:ConcentrationofH2O2was9.794mmol·L-1.InitialconcentrationofFe2+was2.4485mmol·L-1.InitialpHvaluewas3.5.Thereactiontimewas45min.Highsalinitywouldresultinlowreductionrateof TOC.IfflocculationPDADMACwasadded,thereductionratewas54.68%whichwas notquitesatisfactoryandneededimproving.Theresearchwasalsoputintotreatingsecondarysedimentationtanksewagefromacertainchemicalparkplant.Thebestoperatingconditionwere:ConcentrationofH2O2was7.346mmol·L-1.Initialconcentrationof Fe2+was0.9182mmol·L-1.Thereactiontimewas90min.Undertheoptimalcondition,reductionrateofTOCwas45.64%.ComparedwithCPAM,PDADMAChadtheadvantageoflessamountusedandahigherTOCreductionrate.SoPDADMACwasselected.TheoptimalinputforPDADMACwas2mg·L-1.Andreductionrateof TOCwas54.68%.Afterthetreatment, thewatercouldstrictlymeettherequirementofeffluentstandardoflevel2.Keywords:Fenton,Flocculation,PFOS,Hydroquinone,AdvanceTreatment目录独创性声明............................................................................................................... I摘要...............................................................................