利用光子回波分析尼尔蓝分子的电子态振动模式及其弛豫过程-analysis of electronic vibration modes and relaxation processes of neil blue molecules by photon echo.docxVIP

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利用光子回波分析尼尔蓝分子的电子态振动模式及其弛豫过程-analysis of electronic vibration modes and relaxation processes of neil blue molecules by photon echo.docx

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利用光子回波分析尼尔蓝分子的电子态振动模式及其弛豫过程-analysis of electronic vibration modes and relaxation processes of neil blue molecules by photon echo

AbstractAlong with the advent of femtosecond laser pulse, the research about three-pulse photon echo become more and more widely. Scientists probe the liquid ultrafast dynamic process and line broadening of the electronic transition through photon echo. This paper takes Nile blue as sample, studying the three-pulse photon echo from theory and experiment respectively.Using the optical bloch equation to calculate the bloch vectors in the process of optical nutation and optical free induction decay. Analysing the three-pulse photon echo through the optical nutation and the optical free induction decay. With the Maxwell wave equation, we build the relationship between the intensity of three-pulse photon echo signal and the bloch vectors. In this paper, we treat the vibration of material molecules as the model of the Multimode Brownian Oscillator, and discuss that how to calculate the three-pulse photon echo signal. Taking the Nile blue for example, we use the model of the Multimode Brownian Oscillator to analyse the vibration of the Nile blue molecules and regard the vibration of the Nile blue molecules as the weighted coupling result of the gaussian, overdamping, completely inhomogeneous, underdamping model. Changing the weight of these four model to alter the correlation function of the Nile blue molecules, we numerically simulate the three-pulse photon echo signal, the transient grating photon echo signal and the three-pulse photon echo peak shift.During the experiment research about the three-pulse photon echo of the Nile blueethanol solution, the concentration of Nile blue ethanol solution is8?10?5 mol / L , thewavelength and the pulse width of the femtosecond laser light source are 623nm and 40fs respectively. We divide the femtosecond laser light source into three beams and the power of each beam pulse is 20uw. On the basis of that these three femtosecond laser pulses are completely overlap both in space and time, we measure the three-pulse photon echo signal of