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Using coherent xrays to study the dynamics of condensed matter 利用相干X射线来的研究凝聚态动力学
* * * * * * * * * Conclusions XPCS will benefit tremendously from a new generation of coherent x-ray sources, because brightness determines the XPCS SNR. Be aware, however, that the single most important way to improve XPCS today -- and absolutely required at sources with 5000-fold improved brightness -- is with improved x-ray detectors. Overall, we are behind where we should be w.r.t. x-ray area detectors and behind European detector efforts (e.g. Medipix, Pilatus) Conclusions (cont.) Desirable XPCS detector characteristics include: High speed (determines the fastest processes that can be studied.) High efficiency at high x-ray energy. (High x-ray energy minimizes sample damage.) Large number of pixels. (Can be increased with multiple detectors.) Small pixel size to (nearly) resolve speckles. On-pixel correlation, in order to circumvent issue of the tremendous data rate for a framing camera. Conclusions (cont.) Conclusions (cont.) For many soft matter experiments, it will be essential to address the issue of sample damage right from the start. Fortunately, to make meaningful XPCS measurements, it is necessary to illuminate for only a few times the (slowest) correlation time. This indicates a sample flow/translation scheme that effectively moves a new sample into the beam on a time scale slow compared to the correlation time, and fast compared to the damage time. Thanks to: Xinhui Lu (Yale) Peter Falus (Yale/MIT/ILL) Michael Sprung (APS) Alec Sandy (APS) Suresh Narayanan (APS) THE END * * * * * * * * * * * * * * * * * * * * * * * * * * * Using coherent x-rays to study the dynamics of condensed matter Simon Mochrie, Yale University Outline What is x-ray photon correlation spectroscopy (XPCS)? Why coherent x-ray beams and brightness? Example 1:Glass transitions in a colloidal suspension with tunable attractions. Example 2: Dynamics of polymer membranes. Example 3: Near-field heterodyne speckle. Prospects, Comments and Conclusions What is XPCS? XPCS is a meth
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