Investigation of Coherent-Control cont#39;d - Yale University相干控制、管理和# 39调查；D -耶鲁大学.pptVIP

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Investigation of Coherent-Control cont#39;d - Yale University相干控制、管理和# 39调查；D -耶鲁大学.ppt

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InvestigationofCoherent-Controlcont

Photo-Excitation and Relaxation Processes Aspects of Study Interfacial Electron Transfer Dynamics Relevant timescales and mechanisms Total photo-induced current Dependence of electronic dynamics on the crystal symmetry and dynamics Hole Relaxation Dynamics Decoherence timescale. Effect of nuclear dynamics on quantum coherences, coherent-control and entanglement. Model System – Unit Cell TiO2-anatase nanostructure functionalized by an adsorbed catechol molecule Mixed Quantum-Classical Dynamics Propagation Scheme Time-Dependent Propagation Scheme cont’d Time-Dependent Propagation Scheme cont’d Model System – Mixed Quantum-Classical Simulations LUMO Injection (frozen lattice) cont’d Reduced Density Matrix: Hole-States Occupancy Notation Investigation of Entanglement cont’d Investigation of Coherences cont’d Investigation of Coherences cont’d Investigation of Coherences cont’d Investigation of Coherences cont’d Decoherence Dynamics cont’d Off-diagonal elements are indicative of decoherence if nuclear motion randomizes the phases, i.e, becomes a random quantity and the average The system will no longer be in a coherent superposition of adsorbate states. Diagonal Elements of the Reduced Density Matrix T=100 K Off-Diagonal Elements of the Reduced Density Matrix T=100 K Time, ps Time, ps Measure of decoherence: + + + + 100 fs * * Mr. Sabas Abuabara Sabas Abuabara, Luis G.C. Rego and Victor S. Batista Department of Chemistry, Yale University, New Haven, CT 06520-8107 Quantum Information and Quantum Control Conference July 19-23, 2004 - University of Toronto, The Fields Institute, Toronto (BA1170) Dr. Luis G.C. Rego* *Current Address: Physics Department, Universidade Federal do Parana, CP 19044, Curitiba, PR, Brazil, 81531-990 Creating and Manipulating Electronic Quantum Coherences in Functionalized Semiconductor Nanostructures Add energy diagram here Interfacial electron transfer Hole relaxation dynamics Luis G.C. Rego and Victor S. Bat