大气化学-7-氮循环.pptVIP

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大气化学-7-氮循环.ppt

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* 4.5.5 模式计算例子(大气氮） A global modelling study of the atmospheric nitrogen budgetJér?me DrevetIsabelle Bey * HNO3 NO 3 - N2 NO NH3/NH4+ NH3/NH4+ NO2 OrgN Primary emissions Decay Assimilation Nitrification Denitrification Deposition Fixation Lightning Fertilizer Deposition Fixation Fixation Assimilation N2O Oxidation Nitrogen cycle NOy = NOx + NO3 + HNO2 + N2O5 + PAN NHx = NH3 + NH4+ * Assimilated Meteorological Fields [NASA-DAO] . 20 to 50 ?-layers . Surf to 10-0.01 hPa . 4°x5°, 2°x2.5°, 1°x1° . every 3-6 hours . data from 1988 . data : U,V,P,T, water content, insolation @ ground cloud cover, fraction, optical depth, etc Transport algorithms: Advection, Convection, Boundary Layer Mixing [Allen et al., 1996; Lin Rood, 1996] Chemical solver [Wang et al., 1998] Photolysis [Wild et al., 2000] GEOS-CHEM 3-D Ox-NOx-Hydrocarbon chemistry Sulfate-nitrate-ammonium aerosols [Bey et al., 2001; Martin et al., 2002] Aerosol Fields . Dusts . Sea-salts . Black Carbon . Organic Carbon [Chin et al., 2002; Ginoux et al., 2002; Martin et al., 2002] Inventories for fossil fuel, biomass burning, biofuel [J. Logan; Duncan et al., 2002] Algorithms for biogenic emissions [Wang et al., 1998] Algorithms for lightning emissions [Price and Rind, 1992; Pickering et al., 2001] Upper (stratospheric) boundary conditions [McLinden et al., 2000] Dry Wet Deposition [Wang et al., 1998; Liu et al., 2000] 3-D model of chemistry/transport * EMEP observations GEOS-CHEM results EMEP : European Monitoring and Evaluation Program Model evaluation 2: NH4+ deposition Too coarse resolution * Atmosphere N budget 1: Total N deposition * Total N emissions (TgN/yr): Total N deposition (TgN/yr): Atmospheric N budget 2: Comparison with previous works (holland et al. [1997]) * * * * Here we evaluate ammonia deposition using NH4+ wet deposition measurements from EMEP network * We present here the total N budget obtained with GC in comparison with previous model results. We can see that our model