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ResearchArticle

Visible-Light-ActivePlasmonicAg−SrTiO3Nanocompositesforthe

DegradationofNOinAirwithHighSelectivity

QianZhang,†YuHuang,*,†,‡LifengXu,†Jun-jiCao,*,†,‡WingkeiHo,§andShunChengLee∥

†KeyLaboratoryofAerosolChemistryandPhysics,InstituteofEarthEnvironment,ChineseAcademyofSciences,Xi’an710061,

China

‡StateKeyLabofLoessandQuaternaryGeology(SKLLQG),InstituteofEarthEnvironment,ChineseAcademyofSciences,Xi’an

710061,China

§DepartmentofScienceandEnvironmentalStudies,TheHongKongInstituteofEducation,HongKong,China

∥DepartmentofCivilandEnvironmentalEngineering,TheHongKongPolytechnicUniversity,HungHom,HongKong,China

S

*SupportingInformation

ABSTRACT:Harnessinginexhaustiblesolarenergyforphotocatalyticdisposalofnitrogenoxidesisofgreatsignificance

nowadays.Inthisstudy,Ag−SrTiO3nanocomposites(Ag−STO)weresynthesizedviaone-potsolvothermalmethodforthefirst

time.ThedepositionofAgnanoparticlesincursabroadplasmonicresonanceabsorptioninthevisiblelightrange,resultingin

enhancedvisiblelightdrivenactivityonNOremovalincomparisonwithpristineSrTiO3.TheAgloadingamounthasa

significantinfluenceonlightabsorptionpropertiesofAg−STO,whichfurtheraffectsthephotocatalyticefficiency.Itwasshown

that0.5%AgloadingontoSrTiO3(inmassratio)couldremove30%ofNOinasinglereactionpathundervisiblelight

irradiation,whichistwicehigherthanthatachievedonpristineSrTiO3.Mo