Bandgap Engineering in ZnO By Doping with 3d Transition Metal Ions英文文献资料.docVIP

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Bandgap Engineering in ZnO By Doping with 3d Transition Metal Ions英文文献资料.doc

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Bandgap Engineering in ZnO By Doping with 3d Transition Metal Ions英文文献资料

HindawiPublishingCorporation JournalofAtomic,Molecular,andOpticalPhysics Volume2011,ArticleID270540,7pages doi:10.1155/2011/270540 ResearchArticle BandgapEngineeringinZnOByDopingwith 3dTransitionMetalIons D.PaulJoseph1,2andC.Venkateswaran1 1 2 MaterialsScienceCentre,DepartmentofNuclearPhysics,UniversityofMadras,GuindyCampus,Chennai600025,India CenterforCondensedMatterSciences,NationalTaiwanUniversity,Taipei10617,Taiwan CorrespondenceshouldbeaddressedtoC.Venkateswaran,cvunom@ Received6November2010;Accepted21February2011 AcademicEditor:RobertMoshammer Copyright?2011D.P.JosephandC.Venkateswaran. This is an open access article distributed under the Creative Commons AttributionLicense,whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkis properlycited. inBulktheirZn0band.95TMgap0.05Oenergies(TM=Cr,usingMn,DiFe,?useCo,Re?ectanceandNi)wereSpectroscopysynthesizedinbythethestandardultraviolet-visibleceramicmethodregion.andPhaseexploredquanti?cationforvariationand compositionalstudieswereperformedusingRietveldanalysisoftheX-RayDi?ractionpatterns,ScanningElectronmicroscopy, andEnergyDispersiveX-RayAnalysis.Dueto3dtransitioniondoping,thesampleshavebrilliantcolors,andtheabsorptionedge ofZn0.95TM0.05Owasfoundtoshifttowardsthevisibleandultraviolet-visibleregion.Theblueandredshiftsinbandgapsobserved forvarioustransitionmetalion-dopedZnOarediscussed. 1.Introduction transition metal ions apart from introducing spin degree offreedomintotheZnOmatrix.Bandgaptailoringatthe ultravioletendandvisibleregionofthesolarspectrumisof considerableinterestforlargeareaopticalcoatings.Asmost oftheopticalstudiesonZnODMSwereonthin?lmsonly, the present study is aimed at measuring directly the band gapenergiesofbulkZn0.95TM0.05O(TM=Cr,Mn,Fe,Co, Ni) using Di?use Re?ectance Spectrocopy (DRS) which isparticularlysuitableforthedeterminationofabsorption edgesofpowderedmaterials.BulkZn0.95TM0.05O(TM=Cr, Mn,Fe,CoNi)preparedbyceramicmethodwereexplored fortheirstructura