Uncertainty in techno-economic estimates of cellulosic ethanol production due to experimental measurement uncertainty 英文参考文献.docVIP
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Uncertainty in techno-economic estimates of cellulosic ethanol production due to experimental measurement uncertainty 英文参考文献
Vicarietal.BiotechnologyforBiofuels2012,5:23
/content/5/1/23
RESEARCH
OpenAccess
Uncertaintyintechno-economicestimatesof
cellulosicethanolproductionduetoexperimental
measurementuncertainty
KristinJVicari1,2,SaiSandeepTallam1,2,TatyanaShatova1,2,KohKangJoo1,2,ChristopherJScarlata3,
DavidHumbird3,EdwardJWolfrum3*andGreggTBeckham3,4*
Abstract
Background:Cost-effectiveproductionoflignocellulosicbiofuelsremainsamajorfinancialandtechnicalchallenge
attheindustrialscale.Acriticaltoolinbiofuelsprocessdevelopmentisthetechno-economic(TE)model,which
calculatesbiofuelproductioncostsusingaprocessmodelandaneconomicmodel.Theprocessmodelsolvesmass
andenergybalancesforeachunit,andtheeconomicmodelestimatescapitalandoperatingcostsfromthe
processmodelbasedoneconomicassumptions.Theprocessmodelinputsincludeexperimentaldataonthe
feedstockcompositionandintermediateproductyieldsforeachunit.Theseexperimentalyielddataarecalculated
fromprimarymeasurements.Uncertaintyintheseprimarymeasurementsispropagatedtothecalculatedyields,to
theprocessmodel,andultimatelytotheeconomicmodel.Thus,outputsoftheTEmodelhaveaminimum
uncertaintyassociatedwiththeuncertaintyintheprimarymeasurements.
Results:WecalculatetheuncertaintyintheMinimumEthanolSellingPrice(MESP)estimateforlignocellulosic
ethanolproductionviaabiochemicalconversionprocess:dilutesulfuricacidpretreatmentofcornstoverfollowed
byenzymatichydrolysisandco-fermentationoftheresultingsugarstoethanol.Weperformasensitivityanalysison
theTEmodelandidentifythefeedstockcompositionandconversionyieldsfromthreeunitoperations(xylosefrom
pretreatment,glucosefromenzymatichydrolysis,andethanolfromfermentation)asthemostimportantvariables.
Theuncertaintyinthepretreatmentxyloseyieldarisesfrommultiplemeasurements,whereastheglucoseand
ethanolyieldsfromenzymatichydrolysisandfermentation,respectively,aredominatedbyasinglemeasurement:
thefractionofinsolublesolids(fIS)inthebiomassslurries.
Conclusions:Wecalculatea$0.15/galuncertaintyinMESPfromtheTEmodelduetouncertaintiesinprim
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