原创力文档electrodeposition of platinum and ruthenium nanoparticles in multiwalled carbon nanotube-nafion nanocomposite for methanol electrooxidation电沉积铂和钌纳米颗粒的微碳nanotube-nafion甲醇电氧化的纳米复合材料.pdfVIP
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electrodeposition of platinum and ruthenium nanoparticles in multiwalled carbon nanotube-nafion nanocomposite for methanol electrooxidation电沉积铂和钌纳米颗粒的微碳nanotube-nafion甲醇电氧化的纳米复合材料
Hindawi Publishing Corporation
Journal of Nanomaterials
Volume 2009, Article ID 892178, 6 pages
doi:10.1155/2009/892178
Research Article
Electrodeposition of Platinum and Ruthenium Nanoparticles in
Multiwalled Carbon Nanotube-Nafion Nanocomposite for
Methanol Electrooxidation
Yu-Huei Hong and Yu-Chen Tsai
Department of Chemical Engineering, National Chung Hsing University, 250 Kuo Kuang Road, Taichung 40227, Taiwan
Correspondence should be addressed to Yu-Chen Tsai, yctsai@.tw
Received 27 May 2009; Accepted 25 August 2009
Recommended by Zhi-Li Xiao
PtRu nanoparticles with a diameter of 10–15 nm were electrodeposited within multiwalled carbon nanotube-Nafion (MWCNT-
Nafion) nanocomposite. The formation of PtRu nanoparticles in MWCNT-Nafion nanocomposite was characterized by scanning
electron microscopy, transmission electron microscopy, and energy dispersive X-ray spectroscopy. The electrocatalytic activity
towards the methanol electrooxidation at PtRu-MWCNT-Nafion and Pt-MWCNT-Nafion nanocomposite-modified glassy
carbon electrodes was investigated by cyclic voltammetry. The results indicated that the PtRu-MWCNT-Nafion nanocomposite
was electrocatalytically more active than Pt-MWCNT-Nafion nanocomposite. The effect of atomic ratio of Pt : Ru on the
electrocatalytic ability towards the methanol electrooxidation was investigated in order to achieve a high catalyst use. The PtRu
bimetallic catalyst with 1 : 1 atomic ratio showed better electrocatalytic activity towards the methanol electrooxidation. The
stability for the methanol electrooxidation at PtRu-MWCNT-Nafion nanocomposite modified was also investigated.
Copyright © 2009 Y.-H. Hong and Y.-C. Tsai. This is an open access article distributed under the Creative Commons A
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