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direct decomposition of no into n2 and o2 over c-type cubic y2o3-tb4o7-zro2没有直接分解成n2和o2 c -型立方y2o3-tb4o7-zro2
Materials Sciences and Applications, 2012, 3, 733-738
/10.4236/msa.2012.310107 Published Online October 2012 (http://www.SciRP.org/journal/msa)
Direct Decomposition of NO into N and O over C-Type
2 2
Cubic Y O -Tb O -ZrO
2 3 4 7 2
*
Toshiyuki Masui, Shunji Uejima, Soichiro Tsujimoto, Nobuhito Imanaka
Department of Applied Chemistry, Faculty of Engineering, Osaka University, Suita, Japan.
*
Email: imanaka@chem.eng.osaka-u.ac.jp
Received July 14th, 2012; revised August 15th, 2012; accepted September 16th, 2012
ABSTRACT
Catalytic activities for direct NO decomposition were investigated over C-type cubic Y O -Tb O -ZrO prepared by a
2 3 4 7 2
co-precipitation method. The NO decomposition activity was enhanced by partial substitution of the yttrium sites with
terbium in a (Y Zr ) O catalyst, which shows high NO decomposition activity. Among the catalysts synthesized
0.97 0.03 2 3.03
in this study, the (Y Tb Zr ) O catalyst exhibited the highest NO decomposition activity; NO conversion to N
0.67 0.30 0.03 2 3.33 2
was as high as 67% at 900˚C in the absence of O2 (NO/He atmosphere), and a relatively high conversion ratio was ob-
served even in the presence of O or CO , compared with those obtained over conventional direct NO decomposition
2 2
catalysts. These results indicate that the C-type cubic Y O -Tb O -ZrO catalyst is a
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