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quantum dot sensitized photoelectrodes量子点敏化光电极
Nanomaterials 2011, 1, 79-88; doi:10.3390/nano1010079
OPEN ACCESS
nanomaterials
ISSN 2079-4991
/journal/nanomaterials
Review
Quantum Dot Sensitized Photoelectrodes
Thomas J. Macdonald and Thomas Nann *
Ian Wark Research Institute, University of South Australia, Adelaide, SA 5095, Australia;
E-Mail: tom.macdonald@.au
* Author to whom correspondence should be addressed; E-Mail: thomas.nann@.au;
Tel.: +61-8-8302-5369; Fax: +61-8-8302-3683.
Received: 18 October 2011 / Accepted: 26 October 2011 / Published: 15 November 2011
Abstract: Quantum Dots (QDs) are promising alternatives to organic dyes as sensitisers
for photocatalytic electrodes. This review article provides an overview of the current state
of the art in this area. More specifically, different types of QDs with a special focus on
heavy-metal free QDs and the methods for preparation and adsorption onto metal oxide
electrodes (especially titania and zinc oxide) are discussed. Eventually, the key areas of
necessary improvements are identified and assessed.
Keywords: Quantum dots; dye-sensitized photoelectrodes; photocatalysis; solar energy
conversion; titania; zinc oxide
1. Introduction
Dye sensitized photoelectrodes (e.g., electrodes coated with a photocatalyst) form the basis of many
exciting applications such as solar powered energy conversion (artificial photosynthesis) [1,2]
self-cleaning glass [3], sterilisation [4], and others. In these applications, a dye is exci
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