变气压脉冲放电等离子体发展特性的分析-analysis of development characteristics of variable pressure pulsed discharge plasma.docx

的电子能量变化趋势，随气压升高迅速降低。4．研究了不同气压下，氮气、空气脉冲放电的发展特性。（i）气压在 10~200Pa， 不同的气体放电的发展具有相似性，推进速度均在 107m/s 量级。可通过公 式vde =—2eE λ e 估算放电头部中电子的漂移速度，在气压低于 1000Pa 的气体放电中，mevde 计算值与实验值基本一致。（ii）氮气气压高于 1000Pa，氮气放电迅速减弱。（iii）空气放电中由于氧气的电负性特性，在 1000Pa-1500Pa 之间，放电的发展过程出现 三个阶段：等离子体段推进阶段，等离子体段分离子弹的阶段，等离子体段悬浮放 电，子弹继续推进的阶段。5．高气压下脉宽对放电发展影响很大。气压在 5×103Pa~104Pa 之间，脉宽占空 比 20%~90%时，在管内静止气体中产生等离子体射流。射流最长达到 30cm，放电 也是以等离子体子弹的形式发展，与大气压等离子体射流的发展特性基本一致。当 脉宽占空比介于 60%~90%之间，射流出现亮暗分段现象。长脉宽下，正离子（氩气 中主要是氩离子）在弱电场中的长时间迁移运动，以及激发态粒子在弱电场中的反 应过程对放电的影响，可能是产生射流以及射流亮暗分段的原因。关键词：脉冲放电；放电发展特性；快速电离波； 等离子体段；等离子体子弹；电子激发温度AbstractNon-equilibrium plasmas generated by pulsed DC discharge have an electron temperature that is much higher thangas temperatureat low, moderate and atmospheric pressure. Owing to some unique technical advantages of the pulsed plasmas, they have come to play an increasing rolein many novel applications, such as biological and chemical decontaminations of media, surface modification/functionalization of polymers,deposition of thin films, the synthesisof carbon nanotubes,productionof graphene-based materials, absorption and reflection ofelectromagnetic waves,etc. Although the propagation Characteristics of the pulsed discharge has been studied for decades, some peculiar phenomena depends on many experimentalconditions and the nature of the dependences on theseconditions is not yet known sufficiently well for reliableextrapolations.As working medium of gas discharge, gas has a direct effect on the characteristics of discharge. In this dissertation, effects of gas pressure and gas composition on discharge are investigated, and the details are presented as follows:1．A DBD system which can exactly control the gas pressure and composition wasconstructed.2．The transition of propagation mode depended on gas pressure was studied with an high speed ICCD camera. (i) Pressure between 10Pa~200Pa, fast ionization wave (FIW) discharge is generated in the tube by pulse voltage (amplitude 7kV, frequency 4kHz, and pulse