超短脉冲激光激发下双光子吸收系数的研究-理论物理专业论文.docxVIP

超短脉冲激光激发下双光子吸收系数的研究 超短脉冲激光激发下双光子吸收系数的研究 STUDY ON THE TWO-PHOTON ABSORPTION COEFFICIENT UNDER THE EXCITATION OF ULTRA-SHORT PULSE LASER ABSTRACT The study dealing with the two-photon absorption (TPA) properties of materials induced by ultra-short pulse laser is one of the hotspots in Optoelectronics field. The molecular TPA cross section (σ2) is a well known parameter which can describe importantly the TPA properties of media. The σ2 value of some medium can be experimentally obtained by way of measuring two-photon absorption coefficient (β). There are many methods to obtain β experimentally, such as nonlinear transmission, Z-scan, and two-photon induced fluorescent comparison. The actual quantity typically measured in nonlinear transmission and Z-scan is energy transmission, which depends on not only the TPA coefficients but also the pulse profile of laser. Since it is usually a hard task to give a precise description of the ultra-short pulse envelope of a used laser, some pulse model has to be assumed in the TPA performance. As a result, for a set of experimental data of energy transmission, the different values of β will be obtained based on different pulse models. The main purpose of this paper is to attempt to give out the quantitative β differences resulting from the applications of some typical ultra-short pulse models. These results may be helpful to obtain, in experimental principle, an exact β of a nonlinear medium in the datum process of TPA measurement. Based on the typical ultra-short pulse models, such as rectangular, Gaussian, sech2, Lorentz, and asymmetric sech2, we have studied the relation between nonlinear energy transmission and ultra-short pulse spatial and temporal structure by way of numerical simulation and theoretically, respectively. Our mainly academic achievements are following. ii 河北工业大学硕士学位论文 河北工业大学硕士学位论文 We first obtain the difference curves of nonlinear energy transmissions for the five ultra-short pulse models. In addition, the relati