激光相干控制.pptx

Laser control of product quantum state populations in unimolecular reactions;Outline;Background ;Theory and experiment;Theory and experiment;Theory and experiment; Experimentally altering and x, which include phase and amplitude effects due to both the superposition state preparation and subsequent applied fields, provides control over the probability of observing the (q,n) product state. For example: ;Theory and experiment;Theory and experiment; The quantum state yield, in case (a), is seen to be controllable over a range of 0%-20% whereas a 0%-2% range is possible in case (b). The maximum yield, in both cases, is substantially larger than the single laser configuration (S = 0 or S = 1); The approach advocated in this Communication suggests a wide range of theoretical and experimental applications in state preparation and control of unimolecular reactions.