石墨烯基阴极电催化材料的理论设计与制备-化学工程专业毕业论文.pdfVIP

石墨烯基阴极电催化材料的理论设计与制备 Theoretical Design and Experimental Synthesis of Graphene-based Cathode Electrocatalytic Materials Abstract Currently the two major problems facing humanity are energy shortage and environmental pollution．Development and utilization of new，high efficiency and clean energy resources iS the inevitable choice for sustainable development．Dye·sensitized solar cells(DSCs)have been drawing wide-spread attention because of their lOW cost ， environmental friendliness，the dye availability，their easy fabrication，and their high power conversion efficiency(PCE)．To date．ceaified champion efficiency of more than l 4％has been achieved．which has a good industrial prospects．Fuel cell(FCs)，a clean and efficient power generation device that Can directly convea the chemical energy of the fuel into electrical energy，have shown some excellent advantages such as high energy conversion efficiency．broad source and litter pollution to environmental．Cathodic electrocatalytic reduction reaction is the key to research and develop of these two new energy devises． Traditionally．noble metal Platinum has been widely used as a cathode materials in DSCs and FCs due to its high catalytic activity and high electronic conductivity．However，because of high cost，lOW abundance in nature，poor stability in corrosive electrolytes，and easily dissolved in the electrolyte solution，using Pt presents major drawbacks for large—scale production ofDSCs and FCs．Finding alternative materials to Pt with lowmanufacturing cost and high electrocatalytic activity is therefore an important challenge．The aim of this thesis is to design and synthesize high performance graphene based cathode catalysts ． 111e combination of theoretical computation and experiment