填充鼓泡床混合特性的研究.pdfVIP

填充鼓泡床混合特性的研究 摘 要 气液并流向上填充床被广泛地应用到化工、石油化工、环境工程等领域，虽 然近几年对该反应器进行了广泛地研究，但由于体系的复杂性和测量的手段不 同，造成了研究结果的不同。本文在内径为 160mm 气夜并流向上填充塔中，采 用空气和水作为气液体系，研究气液并流向上填充床的流型、压降、轴向返混等 基本流体力学参数。通过目视法观察液体的流型（鼓泡型、脉动型、喷射型）和 用有色颜料作为示踪剂，通过分光光度计测量液体的吸光度，再转化为液体的浓 度以求其平均时间、方差、佩克莱准数等等测试手段。考察了气速、液速和填料 层高度对填充床中液体的返混程度影响。实验得出液相的佩克莱数与气体和液体 的速度有关，主要受气速的影响；填料层越高，液相佩克莱数准数越大。 关键词：并流向上，填充床，佩克莱准数，轴向扩散。 I 填充鼓泡床混合特性的研究 Abstract Numerous chemical processes are carried out in packed bed bubble column reactors with cocurrent upflow of gas and liquid. Extensive studies on the hydrodynamics and mass transfer in packed bed bubble column reactors are reported in literature 。The results have some difference due to the complex of hydrodynamics and the methods. The effects of gas and liquid flow rates and packing height on the liquid phase axial dispersion coefficient and the liquid holdup in a gas-liquid cocurrent upflow packed column with 160mm inner diameter and 1000mm high packing. The flow pattern of liquid (bubble impulse spout) is observed using eyes in the air-water sysytem. The spectrophotometer measures the absorbance using coloured pigment as tracer, and convert it to concentration of liquid to calculate the average time variance and Peclet. The experimental results show the liquid Peclet depends on gas and liquid velocity, and the liquid peclet increases with increasing the packed height. Keywords: cocurrent upflow, Packed bed , Peclet, axial dispersion. II 填充鼓泡床混合特性的研究 目 录 第一章 前言 ………………………………………………………………….…..1 1.1 气液并流向上填充研究的历史