Annealing Effect on Photovoltaic Performance of CdSe Quantum-Dots-Sensitized TiO2 Nanorod Solar Cells英文文献资料.docVIP

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Annealing Effect on Photovoltaic Performance of CdSe Quantum-Dots-Sensitized TiO2 Nanorod Solar Cells英文文献资料.doc

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Annealing Effect on Photovoltaic Performance of CdSe Quantum-Dots-Sensitized TiO2 Nanorod Solar Cells英文文献资料

HindawiPublishingCorporation JournalofNanomaterials Volume2012,ArticleID103417,6pages doi:10.1155/2012/103417 ResearchArticle AnnealingEffectonPhotovoltaicPerformanceofCdSe Quantum-Dots-SensitizedTiO2NanorodSolarCells YitanLi, LinWei, RuiziZhang, YanxueChen, andJunJiao 1 2 1 1 3 1 2 3 SchoolofPhysicsandStateKeyLaboratoryofCrystalMaterials,ShandongUniversity,Jinan250100,China SchoolofInformationScienceandEngineering,ShandongUniversity,Jinan250100,China DepartmentofPhysics,PortlandStateUniversity,P.O.Box751,Portland,OR97207-0751,USA CorrespondenceshouldbeaddressedtoYanxueChen,cyx@ Received4August2012;Revised22October2012;Accepted24October2012 AcademicEditor:JianWei Copyright?2012YitanLietal.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense,which permitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperlycited. Large area rutile TiO2 nanorod arrays were grown on F:SnO2 (FTO) conductive glass using a hydrothermal method at low temperature.CdSequantumdots(QDs)weredepositedontosingle-crystallineTiO2nanorodarraysbyachemicalbathdeposition (CBD)methodtomakeaphotoelectrode.ThesolarcellwasassembledusingaCdSe-TiO2 nanostructureasthephotoanode andpolysul?desolutionastheelectrolyte.Theannealinge?ectonopticalandphotovoltaicpropertiesofCdSequantum-dots- sensitizedTiO2nanorodsolarcellswasstudiedsystematically.Asigni?cantchangeofthemorphologyandaregularredshiftof bandgapofCdSenanoparticleswereobservedafterannealingtreatment.Atthesametime,animprovedphotovoltaicperformance wasobtainedforquantum-dots-sensitizedsolarcellusingtheannealedCdSe-TiO2nanostructureelectrode.Thepowerconversion e?ciency improved from 0.59% to 1.45% as a consequence of the annealing e?ect. This improvement can be explained by consideringthechangesinthemorphology,thecrystallinequality,andtheopticalpropertiescausedbyannealingtreatment. 1.Introduction Considering the high cost and low stability o