Barium Staminate as Semiconductor Working Electrodes for Dye-Sensitized Solar Cells英文文献资料.docVIP

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Barium Staminate as Semiconductor Working Electrodes for Dye-Sensitized Solar Cells英文文献资料.doc

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Barium Staminate as Semiconductor Working Electrodes for Dye-Sensitized Solar Cells英文文献资料

HindawiPublishingCorporation InternationalJournalofPhotoenergy Volume2010,ArticleID105878,7pages doi:10.1155/2010/105878 ResearchArticle BariumStaminateasSemiconductorWorkingElectrodesfor Dye-SensitizedSolarCells Fu-anGuo,GuoqiangLi,andWeifengZhang KeyLaboratoryofPhotovoltaicMaterialsofHenanProvince,SchoolofPhysicsandElectronics, HenanUniversity,Kaifeng475001,China CorrespondenceshouldbeaddressedtoWeifengZhang,wfzhang6@163.com Received2January2010;Revised4April2010;Accepted20April2010 AcademicEditor:DavidLeePhillips Copyright?2010Fu-anGuoetal.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense, whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperlycited. Dye-sensitized solar cells (DSSCs) are fabricated with perovskite-type BaSnO3 as the photoelectrode materials. Di?erent preparation methods including coprecipitation, hydrothermal, and solid state reaction are employed to synthesize BaSnO3 particlestooptimizethephotoelectricactivitiesofelectrodematerials.ThephotoelectricpropertiesofBaSnO3particlesandthe performancesofDSSCsareinvestigatedbysurfacephotovoltagespectroscopyandcurrent-voltagemeasurements.Thelight-to- electricityconversionof1.1%ispreliminarilyreachedontheDSSCmadeofthecoprecipitation-derivedBaSnO3particles.Large currentdensityofholeinjectionintotheHOMOlevelofN719dyefromthevalencebandofBaSnO3andreducedphotogenerated chargerecombinationinBaSnO3couldberesponsiblefortheobservedsolarcellperformanceoftheDSSCfabricatedfromthe coprecipitation-derivedBaSnO3particles. 1.Introduction also be considered and optimized. Perovskite structured BaSnO3 isann-type semiconductingmaterialwithaband gap of 3.1eV [14]. It has been widely investigated on its dielectric, thermal, and photocatalytic properties as an importantceramicmaterial[15].Inthepreviouswork,we have demonstrated that the photogenerated electrons can be injected into the conduction band of BaSnO3 from the excited (Bu4N)2(Ru)(dcbpyH)2(NCS)2