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从Cu2S到Cu(I)掺杂CdS纳米晶的可控离子交换法制备及光学、电学性能研究(英文).pdf
SCIENCE CHINA Materials ARTICLES
Published online 14 September 2015 | doi: 10.1007/s40843-015-0080-z
Sci China Mater 2015, 58: 693–703
From Cu S nanocrystals to Cu doped CdS
2
nanocrystals through cation exchange:
controlled synthesis, optical properties and
their p-type conductivity research
1 1 2 3 4 1 1
Jian Liu , Yuheng Zhao , Jialong Liu , Shouguo Wang , Yan Cheng , Muwei Ji , Yuanmin Zhou ,
1 2 1*
Meng Xu , Weichang Hao and Jiatao Zhang
Heterovalent doping represents an effective method to con- Along this direction, Cu(I) and Ag (I) ions could act as het-
trol the optical and electronic properties of semiconductor erovalent dopants and control both optical and electronic
nanocrystals (NCs), such as the luminescence and electronic impurities properties of II-VI NCs [6–11]. However, the
impurities (p-, n-type doping). Considering the phase struc- common problem to be encountered in the case of Cu-
ture diversity, coordination varieties of Cu atoms in Cu2S NCs,
doped semiconductor NCs is the oxidation state of Cu ions
and complexity of Cu doping in II-VI NCs, monodisperse
Cu2S NCs with pure hexagonal phase were synthesized firstly. and induced stable p-type conductivity [12,13]. Evidence
Then through cation exchange reaction between Cd ions and from several reports showe
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