纳米bifeo3h2o2体系降解染料废水的研究-study on degradation of dye wastewater by nano - bifeo _ 3 h2o2 system.docxVIP

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纳米bifeo3h2o2体系降解染料废水的研究-study on degradation of dye wastewater by nano - bifeo _ 3 h2o2 system.docx

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AbstractWiththerapiddevelopmentofthedyeindustry,effectivedegradationoforganicpollutantsinwastewaterhasbecomeanimportanttopicinenvironmentalgovernance.ClassicFentonreactionhasadvantagesofhighefficiencycatalyticoxidationabilityandnon-toxicharmless,itcandegrademostofthetoxicandhazardoussubstances.However,underacidicconditions(pH3.0),thereactionwascomplete.Generally,theactualpHofwastewaterisinawiderrange,extremelyacidreactionconditionsneedtoaddlargeamountsofacidtoincreasethecostsanddamagestotheenvironment,itsresiduewouldcausesecondarypollutionofwaterbody.Basedontheseproblems,inthispaper,forthepurposeoflookingforefficientmultiphaseFentonreagent,BiFeO3/H2O2systemwasconstructed.Withmalachitegreen,crystalvioletandacidfuchsinastarget,afeasibilitystudyofBiFeO3/H2O2systemfordyewastewatertreatmentwasconducted.Themaincontentisasfollows:ThepreparationofnanoBiFeO3particles.Thesol-gelmethodwasappliedtopreparenano-BiFeO3particles,andsampleswerecharacterizedbyXRDandSEM.Theresultsshowedthatthenano-BiFeO3particleshavealargersurfacearea,strongadsorption,goodparticledispersionuniform,effectivecatalyticactivationofH2O2andeasilyrecoveredandreused,thusBiFeO3/H2O2systemhasgreatpotentialinthedegradationtreatmentofindustrialdyewastewater.SeveralinfluencingfactorsofdegradationofthreedyesusingnanoBiFeO3/H2O2system.Withmalachitegreen,crystalviolet,acidicfuchsinassubstrate,theoptimalreactionconditionsweredeterminedbysinglefactorexperiment.TheresultsshowedthatpHvalue,amountofcatalyst,H2O2volume,initialwastewaterconcentrationandreactiontemperaturehadagreatimpactonthedegradationofthreedyes.WhenthepHvaluewas8.5,8.0,7.5;amountofcatalystwas0.8g/L,0.6g/L,0.45g/L;H2O2volumepercentwas1.00%,0.83%,0.65%;initialconcentrationwas150mg/L,150mg/L,120mg/L;temperaturewas313K,308K,303K;thebestresultsareattained,theremovingratecanreach99%ormore.Thekineticsoftheoxidationdegradationofdyeingwastewaterimitatedwithmalachitegreen,crystalviolet,acidicfuchsinusingnanoBiFeO3/H2O2systemreagentwasstudied.Theeffectsoftheinitialc