纳秒脉冲电源下电晕放电去除苯乙烯-环境工程学报.PDF

第 12 卷　 第 1期 环 境 工 程 学 报 Vol. 12,No. 1 2 0 1 8 年 1 月 Chinese Journal of Environmental Engineering Jan . 2 0 1 8 纳秒脉冲电源下电晕放电去除苯乙烯 刘百良,李驰波,黄逸凡,闫克平,刘振∗ 浙江大学化学工程与生物工程学院,工业生态与环境研究所,杭州 310028 摘　 要　 设计一套纳秒量级的脉冲电源,测试结果表明脉冲上升沿为 15 ns,脉宽 30 ns,输出端串联后最大峰值电压为 20 kV,并联后最大峰值电流为340 A。 电源频率在50 ~600 Hz范围内变化且输出脉冲的极性可调节。 纳秒脉冲源匹配反 应器后产生电晕放电,在相同的电源输出能量下,负脉冲的能量注入效率只有 37.4% ,而正脉冲为 87.3%。 当脉冲频率为 -1 600 Hz 时,反应器功率为59.4 W。 以苯乙烯为目标处理物,当能量密度为 27.4 J ·L 时,苯乙烯降解效率达到 98.6%。 相同能量密度下,负脉冲放电下苯乙烯的去除率最高。 关键词　 低温等离子体;挥发性有机物(VOCs);脉冲电源;苯乙烯 中图分类号　 X511　　 文献标识码　 A　　 文章编号　 1673-9108(2018)01-0145-08　　 DOI　 10.12030/ j.cjee.201706009 Styrene removal using corona discharge combined with nanosecond pulse power supply LIU Bailiang,LI Chibo,HUANG Yifan,YAN Keping,LIU Zhen∗ Industrial Ecological and Environmental Research Institute,College of Chemical and Biological Engineering,Zhejiang University,Hangzhou 310028, China Abstract　 An efficient and reliable pulsed power generator is developed both in circuit principle and design im- plementation. Experimental results show that the rising edge of the pulse is 15 ns,pulse width is 30 ns. The maximum peak voltage is20 kV when the output is connected in series,the maximum peak current after parallel is 340 A. The power supply frequency variesfrom50 to600 Hz and the polarity of the output pulse can be adjus- ted. At the same output energy,the efficiency of negative pulse is only 37.4% ,while positive pulse is87.3%. -1 When the pulse frequency is 600 Hz,the reactor power is 59.4 W. When the energy density is 27.4 J ·L , the degradation efficiency of styrene reaches98.6%. At the same energy density,the removal rate of styrene un- der negative pulse discharge is higher than posi