制备方法对V2O5WO3-TiO2催化剂脱除柴油车尾气中NOx的影响.pdfVIP

ChineseJournalofCatalysis35(2014)2020-2028 催化学报 2014年 第35卷 第12期 1w叭^，．chxb．cn avai1able蠢1www ．sciericed ￡琶lclt eolFn 曩 。 曩蠹 嚣蠢曩 ≮蠢 ～ 。。 。 曩 赫 _ iourna{ho警ag裁、^，w1we Vir o ~cate]~hnj舞 Article EffectofV2Os／WO3-TiOzcatalystpreparationmethodonNOx removalfrom dieselexhaust LeiPang。一，ChiFanaLinaShaoaJunxiaYib，XingCaib，JJanWangb,MingKangb,TaoLia．cJ SchoolofChemistry＆ChemicalEngineering,HuazhongUniversityofScienceandTechnology,Wuhon430074,Hubei,China TechnicalCen~rofDongfengCommercialVehicleCoLtd,Wuhan430056,Hubei,China KeyLaboratory rLargeF‘ormatBatteryMaterialsandSystem,MinistryofEducation，HuazhongUniversiytofScienceandTechnology,Wuhan430074, Hubei,China A R T IC L E JN F 0 A B ST R A C T Articlehistory： V2Os／WO3-Ti02catalystswerepreparedbyconventionalimpregnation (V、ⅣTi-con)andultras- Received20June2014 ound。assistedimpregnationmethods(、n^i-HUST)．Theircaatlyticperformancewastestedforthe Accepted2September2014 selectivecaatlyticreductionfSCR1ofNOwithNH3．TheeffeCtSofthepreparationmethodsonthe Published20December2014 caatlystpropertieswerestudied．ThecaatlystswerecharacterizedbyX-raydiffraction，scanning electronmicroscopy,RamanandX·rayphotoelectronspectroscopy．Bothstructuralinvestigation andNH3-SCRactivityshowedthatthepreparationmethodhadastrongeffectonthethermalbe． Keywords： Selectivecatalyticreduction haviOFoftheV2Os／WO3-TiO2catalysts．Afterahydrothermaltreatment,asignificantlossofN0re— ductionactivitywasobs