CdS-Sensitized ZnO Nanorod Photoelectrodes Photoelectrochemistry and Photoinduced Absorption Spectroscopy英文文献资料.docVIP

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CdS-Sensitized ZnO Nanorod Photoelectrodes Photoelectrochemistry and Photoinduced Absorption Spectroscopy英文文献资料.doc

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CdS-Sensitized ZnO Nanorod Photoelectrodes Photoelectrochemistry and Photoinduced Absorption Spectroscopy英文文献资料

HindawiPublishingCorporation AdvancesinOptoElectronics Volume2011,ArticleID915123,5pages doi:10.1155/2011/915123 ResearchArticle CdS-SensitizedZnONanorod Photoelectrodes:Photoelectrochemistryand PhotoinducedAbsorptionSpectroscopy IdrissBedja CRC,DepartmentofOptometry,CollegeofAppliedMedicalSciences,KingSaudUniversity,Riyadh11433,SaudiArabia CorrespondenceshouldbeaddressedtoIdrissBedja,bedja@.sa Received15June2011;Accepted25July2011 AcademicEditor:SuryaPrakashSingh Copyright?2011IdrissBedja.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense,which permitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperlycited. Thin?lmsofZnOsemiconductornanorods(ZnO-nr)of6μmlengthandthinZnOnanoparticulate?lms(ZnO-np)havebeen preparedandmodi?edwithQ-dotsCdSforcomparisonstudy.PIA(photoinducedabsorptionspectroscopy),amultipurpose toolinthestudyofdye-sensitizedsolarcells,isusedtostudyaquantum-dot-modi?edmetal-oxidenanostrucutredelectrode.Q- dotCdS-sensitizedZnO-nr(1Dnetwork)sensitizedphotoelectrodehasdemonstratedbestperformancesinbothphotoelectrical response(IPCEmax=92%)andbroadeningresponseintofarvisiblecomparingtoZnO-np-basedCdSsolarcell.Preadsorbing ZnO-nrwithZnO-npdoesnotbringfurtherimprovement.TimeconstantforelectroninjectionintoZnO-nrconductionband wasrelativelyfastdecayof6.5ms,similartoTiO2-coatedCdS,andprovesatleastawellpore?llingofZnO-nr?lmbyultra?ne CdSparticles.UnidirectionalelectrontransfermechanisticinZnO-nrhasplayedamajorroleintheseperformances. 1.Introduction generated in the semiconductor remains there and cannot migrate to MO. Thus, the two charges will be separated e?ectively. Dye-sensitizedsolarcells(DSCs)basedonone-dimen- sional(1D)ZnOnanostructures,whichexhibitsigni?cantly higherelectronmobilitythanthatofbothTiO2andZnO-np ?lms[10],haverecentlybeenattractingincreasingattention [10,11]. Incontrastwiththedye-sensitizedsolarcells,fundamen- talunderstandingforthefactorscontrollingtheinterfacial electrontran