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グラフェンの选择的化学修饰による次世代半导体の创出
Annual Report No.28 2014
グラフェンの選択的化学修飾による次世代半導体の創出
Creation of Novel Graphene Semi-Conductors by Selective Chemical Functionalization
H2551
代表研究者 田 原 一 邦 大阪大学 基礎工学研究科 助教
Kazukuni Tahara Assistant Professor, Graduate School of Engineering Science, Osaka University
Development of new methodologies to functionalize graphenes at the nanometer scale is
subject of keen interest for scientists in different research fields because of perspective of various
applications. Among various methodologies, supramolecular assembly provides an attractive
approach to form nanopatterns on graphenes, since many organic molecules is known to form
well-defined patterns on graphitic surfaces via physisorption. Here we show that formations
of two-dimensional (2D) porous molecular networks on single or multi-layered graphenes
fabricated on different substrates by self-assembly of dehydrobenzo[12]annulene (DBA)
derivatives having six alkoxy chains at the interfaces between organic liquid and graphenes.
Scanning tunneling microscopy (STM) and atomic force microscopy (AFM) investigations
revealed that honeycomb networks formed by DBA derivatives are highly flexible and they
follow the topological features of the graphene surfaces without any discontinuity, irrespective
of the step-edges present in the substrate underneath. The investigation on the stability of these
networks confirmed the robustness under ambient air conditions. The robust yet flexible DBA
network formed on graphene surface is a useful platform for further modification of graphene
surface by co-adsorption of other molecular species at the pore and the production of novel
sensor which can recognize targeted molecule.
研究目的
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