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Application of Integer and Fractional Models in Electrochemical Systems英文文献资料.doc

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Application of Integer and Fractional Models in Electrochemical Systems英文文献资料

HindawiPublishingCorporation MathematicalProblemsinEngineering Volume2012,ArticleID248175,17pages doi:10.1155/2012/248175 ResearchArticle Application ofIntegerandFractionalModelsin Electrochemical Systems IsabelS.JesusandJ.A.TenreiroMachado Department ofElectricalEngineering, SuperiorInstituteofEngineering ofPorto(ISEP), 4200-072Porto,Portugal Correspondence shouldbeaddressedtoIsabelS.Jesus,isj@isep.ipp.pt Received4July2011;Revised7October2011;Accepted8October2011 Academic Editor:KaticaR.StevanovicHedrih Copyright q2012I.S.JesusandJ.A.TenreiroMachado. This isanopen access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, andreproductioninanymedium,providedtheoriginalworkisproperlycited. This paper describes the use of integer and fractional electrical elements, for modelling two electrochemical systems.A?rsttypeofsystemconsistsofbotanicalelements andasecondtypeis implemented byelectrolyteprocesseswithfractalelectrodes.Experimental resultsareanalyzed in thefrequency domain, andthe prosand cons ofadopting fractional-order electrical components formodelling thesesystemsarecompared. 1.Introduction FractionalcalculusFCisageneralizationoftheintegrationanddi?erentiationtoanonin- tegerorder.Thefundamentaloperatoris aDα,wheretheorderαisarealoreven,acomplex t numberandthesubscriptsaandtrepresentthetwolimitsoftheoperation1–8. RecentstudiesbroughtFCintoattentionrevealingthatmanyphysicalphenomenacan bemodelledbyfractionaldi?erentialequations9–17.Theimportanceoffractional-order modelsisthattheyyieldamoreaccuratedescriptionandleadtoadeeperinsightintothe physicalprocessesunderlyingalong-rangememorybehavior. Capacitorsareoneofthecrucialelementsinintegratedcircuitsandareusedexten- sivelyinmanyelectronicsystems18.However,Jonscher19demonstratedthattheideal capacitorcannotexistinnature,becauseanimpedanceoftheform1/jωCwouldviolate causality 20, 21. In fact, the dielectric materials exhibit