Apparent Enhanced Solubility of Single-Wall Carbon Nanotubes in a Deuterated Acid Mixture英文文献资料.docVIP

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Apparent Enhanced Solubility of Single-Wall Carbon Nanotubes in a Deuterated Acid Mixture英文文献资料.doc

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Apparent Enhanced Solubility of Single-Wall Carbon Nanotubes in a Deuterated Acid Mixture英文文献资料

HindawiPublishingCorporation ResearchLettersinNanotechnology Volume2008,ArticleID296928,4pages doi:10.1155/2008/296928 ResearchLetter ApparentEnhancedSolubilityofSingle-WallCarbon NanotubesinaDeuteratedAcidMixture T.Ramanathan,1FrankT.Fisher,2RodneyS.Ruoff,3andL.CatherineBrinson1,4 1 2 3 4 DepartmentofMechanicalEngineering,NorthwesternUniversity,Evanston,IL60208,USA DepartmentofMechanicalEngineering,StevensInstituteofTechnology,Hoboken,NJ07030,USA DepartmentofMechanicalEngineering,TheUniversityofTexasatAustin,Austin,TX78712,USA DepartmentofMaterialsScienceandEngineering,NorthwesternUniversity,Evanston,IL60208,USA CorrespondenceshouldbeaddressedtoFrankT.Fisher,?sher@ Received8January2008;Accepted17March2008 RecommendedbyValeryN.Khabashesku Anapparentenhancedsolubilityofsingle-wallcarbonnanotubes(SWNTs)inthedeuteratedformofthestandard3:1sulfuric (H2SO4)tonitric(HNO3)acidmixturetreatmentisreportedandattributedtothestrongerinteractionofdeuteriumbondswith thesingle-wallcarbonnanotubesurface.UV-Visiblespectroscopywasusedtocharacterizetheapparentenhancedsolubilityof theSWNTstreatedindeuteratedformsoftheacidmixtureincomparisontothestandardacidmix,whileFTIRwasusedto analyzethenatureofthefunctionalgroupsgeneratedontheSWNTsasaresultofthedi?erentacidtreatments.Theapparent enhancedsolubilityreportedhereisconsistentwiththelimitednumberofcomputationalandexperimentalresultspublishedin theliteratureregardingtheinteractionofcarbonnanotubeswithdeuteratedsolvents;however,adetailedunderstandingofthe underlyingmechanismresponsibleforthisobservationiscurrentlylacking.Theapparentincreasedsolubilityobservedherecould potentiallybeutilizedinmanyapplicationswherecarbonnanotubedispersionisrequired. Copyright?2008T.Ramanathanetal.ThisisanopenaccessarticledistributedundertheCreativeCommonsAttributionLicense, whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperlycited. 1. INTRODUCTION whichwewillrefertoastheD-acidmixture)resultsinanap- parent signi?