Application of Thermosensitive Peptide Copolymer Gels to Removal of Endocrine Disruptor英文文献资料.docVIP

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Application of Thermosensitive Peptide Copolymer Gels to Removal of Endocrine Disruptor英文文献资料.doc

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Application of Thermosensitive Peptide Copolymer Gels to Removal of Endocrine Disruptor英文文献资料

HindawiPublishingCorporation ResearchLettersinMaterialsScience Volume2009,ArticleID597308,4pages doi:10.1155/2009/597308 ResearchLetter ApplicationofThermosensitivePeptideCopolymerGelsto RemovalofEndocrineDisruptor SatoshiTanimoto,NaotoYagi,andHitoshiYamaoka DepartmentofMaterialsScience,TheUniversityofShigaPrefecture,Hassaka,Hikone522-8533,Japan CorrespondenceshouldbeaddressedtoSatoshiTanimoto,tanimoto@mat.usp.ac.jp Received22April2009;Accepted2July2009 RecommendedbyPeterMajewski Poly(L-leucine)-block-poly(ethylene glycol)-block-poly(L-leucine) triblock copolymers were synthesized by a ring-opening polymerizationofα-aminoacidN-carboxyanhydridewithamino-terminatedPEGasaninitiator.Thechloroformsolutionof thesepeptidecopolymersshowedathermo-sensitivesol-geltransition.Thetransitiontemperaturevariedasafunctionofthe lengthofpeptidesegments.Additionally,weusedthesepeptidecopolymerstoremoveanendocrinedisruptorsuchasbisphenol Afromitsaqueoussolution.Asaresult,itbecameclearthatthepeptidecopolymergelusedinthisstudycouldcapturebisphenol Ae?ciently. Copyright?2009SatoshiTanimotoetal. This is an open access article distributed under the Creative Commons Attribution License,whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkisproperly cited. 1.Introduction generativefunctions,andthereforeitisanurgentsubjectto removethemfromtheenvironment[11–13]. Sincethering-openingpolymerizationofα-aminoacidN- carboxyanhydridewaswidelyintroducedbyKricheldorf[1, 2], various type of peptide (poly(amino acid)) has been synthesizedintheworld.Thehistoryofpolymerizationofα- aminoacidN-carboxyanhydridewasdescribedinDeming’s articleindetail[3].Recently,blockcopolymersthatcontain peptide segments are studied eagerly in the various ?elds. For example, the copolymer which consists of two kinds ofpoly(aminoacid)isbeingresearchedforthepurposeof developingstimulusresponsiblematerials[4]. Poly(ethylene glycol) (PEG) is known to have a low toxicityandnottoproduceananti