Application, Evaluation, and Process Analysis of the US EPA’s 2002 Multiple-Pollutant Air Quality Modeling Platform英文文献资料.docVIP

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Application, Evaluation, and Process Analysis of the US EPA’s 2002 Multiple-Pollutant Air Quality Modeling Platform英文文献资料.doc

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Application, Evaluation, and Process Analysis of the US EPA’s 2002 Multiple-Pollutant Air Quality Modeling Platform英文文献资料

Atmospheric and Climate Sciences, 2012, 2, 254-289 /10.4236/acs.2012.23025 Published Online July 2012 (http://www.SciRP.org/journal/acs) Application, Evaluation, and Process Analysis of the US EPA’s 2002 Multiple-Pollutant Air Quality Modeling Platform Kai Wang, Yang Zhang * Department of Marine, Earth, and Atmospheric Sciences, North Carolina State University, Raleigh, USA Email: yzhang9@ * Received May 7, 2012; revised June 1, 2012; accepted June 9, 2012 ABSTRACT A multiple-pollutant version of CMAQ v4.6 (i.e., CMAQ-MP) has been applied by the US EPA over continental US in 2002 to demonstrate the model’s capability in reproducing the long-term trends of ambient criteria and hazardous air pollutants (CAPs and HAPs, respectively) in support of regulatory analysis for air quality management. In this study, a comprehensive model performance evaluation for the full year of 2002 is performed for the first time for CMAQ-MP using the surface networks and satellite measurements. CMAQ-MP shows a comparable and improved performance for most CAPs species as compared to an older version of CMAQ that did not treat HAPs and used older versions of na- tional emission inventories. CMAQ-MP generally gives better performance for CAPs than for HAPs. Max 8-h ozone (O3) mixing ratios are well reproduced in the O3 season. The seasonal-mean performance is fairly good for fine particu- late matter (PM ), sulfate ?SO ? , and mercury (Hg) wet deposition and worse for other CAPs and HAPs species. 2? 4 2.5 The reasons for the model biases may be attributed to uncertainties in emissions for some species (e.g., ammonia (NH3), elemental carbon (EC), primary organic aerosol (POA), HAPs), gas/aerosol chemistry treatments (e.g., secondary or- ganic aerosol formation, meteorology (e.g., overestimate in summer precipitation), measurements (e.g., NO3? ), and the use of a coarse grid resolution. CMAQ cannot well reproduce spatial and seasonal variati