应用全球大气输送模型进行数值模拟研究进展.docVIP

应用全球大气输送模型进行数值模拟研究进展 　　【摘 要】TOMCAT 模型作为多尺度大气输送模型（CTM）的一种，已经在全球范围内得到了广泛应用。大气输送模型是全球温室气体循环研究中一种有效工具，这对于理解全球生态系统的化学循环规律，预测未来气候变化及其对生物多样性的影响具有重要意义。在该模型中，对闪电产生氮氧化物和大气对流过程进行数值模拟是两个重要的因素。为了提高数值模拟的精确性，本文总结了对闪电产生的氮氧化物和大气对流过程进行数值模拟的研究进展，并对将来的研发方向进行了深入探讨。 　　【关键词】环保；TOMCAT模型；大气输送模型；闪电产生氮氧化物；大气对流过程 　　Numerical modeling of lightning produced NOx and convection process in a global chemical transport model （CTM） 　　LIU Huan 　　（Environmental Monitoring Institute of Anyuan Country，Anyuan Jiangxi 342100） 　　【Abstract】The TOMCAT model， as one of CTMs， has been broadly adopted and provides supportive tool to analyze the global circle of greenhouse gas and the chemical dynamics of global ecosystem， which becomes essential for the assessment of climate change effects on biodiversity. In order to improve the simulation accuracy of TOMCAT， this article presents the potential research development（RD） in numerical modeling of both lightning NOx production and convection process on the basis of literature review， both of which significantly influences the distributions of trace gases in CTM. 　　【Key words】Environmental Protection；TOMCAT model；CTM；Lightning NOx production；Convection process 　　0 Introduction 　　TOMCAT model， which simulates the temporal and spatial dynamics of 41 chemical species with a maximum boundary of 10 hPa， is considerably used in atmospheric studies， such as investigation of global greenhouse gas budget （e.g. ozone methane）， study of aviation emission impact on climate（e.g. Kohler et al.， 2008）. So far， there are more than 110 publications based on TOMCAT model since 1993. Tropospheric distributions of trace gases are significantly influenced by meteorological conditions， which include two important processes： convection and associated lightning NOx production（Choi et al.， 2005； Choi et al.， 2008a）. This review presents the potential research development （RD） in simulation of both lightning NOx production and convection for TOMCAT model on the basis of previous