Biologically Inspired Synthesis Route to Three-Dimensionally Structured Inorganic Thin Films英文文献资料.docVIP

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Biologically Inspired Synthesis Route to Three-Dimensionally Structured Inorganic Thin Films英文文献资料.doc

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Biologically Inspired Synthesis Route to Three-Dimensionally Structured Inorganic Thin Films英文文献资料

HindawiPublishingCorporation JournalofNanomaterials Volume2008,ArticleID352871,6pages doi:10.1155/2008/352871 ReviewArticle BiologicallyInspiredSynthesisRoutetoThree-Dimensionally StructuredInorganicThinFilms BirgitSchwenzer1,2andDanielE.Morse1,2,3 1 2 3 InstituteforCollaborativeBiotechnologies,UniversityofCalifornia,SantaBarbara,CA93106-5100,USA CaliforniaNanoSystemsInstitute,UniversityofCalifornia,SantaBarbara,CA93106-5100,USA DepartmentofMolecularCellularandDevelopmentalBiology,UniversityofCalifornia,SantaBarbara, CA93106-9610,USA CorrespondenceshouldbeaddressedtoProf.DanielE.Morse,dmorse@ Received2October2007;Accepted26December2007 RecommendedbyPingXiao Inorganicthin?lms(hydroxide,oxide,andphosphatematerials)thataretexturedonasubmicronscalehavebeenpreparedfrom aqueousmetalsaltsolutionsatroomtemperatureusingvapor-di?usioncatalysis.Thisgenericsynthesisapproachmimicsthe essentialadvantagesofthecatalyticandstructure-directingmechanismsobservedfortheformationofsilicaskeletonsofmarine sponges.Chemicalcomposition,crystallinity,andthethree-dimensionalmorphologyof?lmspreparedbythismethodareex- tremelysensitivetochangesinthesynthesisconditions,suchasconcentrations,reactiontimes,andthepresenceandnatureof substratematerials.Focusingondi?erentmaterialssystems,thereactionmechanismfortheformationofthesethin?lmsandthe in?uenceofdi?erentreactionparametersontheproductareexplained. Copyright?2008B.SchwenzerandD.E.Morse. This is an open access article distributed under the Creative Commons AttributionLicense,whichpermitsunrestricteduse,distribution,andreproductioninanymedium,providedtheoriginalworkis properlycited. 1. INTRODUCTION Biomineralization, including the formation of bones, teeth,shells,orthesilicaskeletonsofmarinesponges,takes placeinvivounderambientconditions.Thesebiomineral- izationprocessesoftenproducehighlyorderedstructureson thenanoscopicaswellasthemacroscopicscale,andgenerally nano-ormicrometer-sizeddefectswithinthesestructuresdo notpropagate,butarecorrectedona