超临界醇热技术制备全波段光催化 复合材料及其性能研究-工业催化专业论文.docxVIP

A Abstract ShanghaiNormalUniversityMaster 万方数据 万方数据 Abstract Photocatalysis has caused great interest in using solar energy to solve environmental pollution problems. As a typical semiconductor, titanium dioxide has attracted lasting concern due to its low toxicity, low cost, excellent chemical stability and high activity. However, as a result of its wide band gap, UV light excitation and low quantum efficiency (QE), the practical application of TiO2 has been prohibited, including pollutants purification, antibacterial and so on. For these reasons, the following three routes were proposed: 1) modifying TiO2 with carbon through novel technique to extend its light absorption edge to visible region. 2) Expanding the applications of photocatalytic materials to purify highly pathogenic bacteria hospital environment, to replace the traditional antibacterial drugs. 3) Designing efficient catalytic reactor to kill bacteria, meeting the needs of practical application. For the above reasons, this graduation thesis mainly includes the following three parts. Supercritical slovothermal route for Ag/TiO2-N with enhanced photocatalytic capability in degrading pollutants. In this section, we prepared Ag/TiO2-N via supercritical solvothermal approach using silver nitrate and tetrabutyl titanate as copper, and titanium source. XRD, SEM and XPS characterizations results showed that supercritical slovothermal treatment resulted in the mesoporous structure, small crystal size, large special surface areas, high crystallinity and high visible-light absorption. Thus, these functional catalysts exhibited high photocatalytic performance and excellent recyclability for MO degradation under visible-light irradiations (λ 420 nm). Research of Ag/TiO2-N photocatalytic antibacterial property of Acimeshobacter baumannii Ag/TiO2-N prepared by the above method used in photocatalytic antibacterial under visible light. In virtue of SEM, ICP and TOC characterizations to study antibacterial process, The